Fast Neutron Reactors
(August 2008)
- Fast neutron reactors are a technological step beyond conventional power reactors.
- They offer the prospect of vastly more efficient use of
uranium resources and the ability to burn actinides which are otherwise
the long-lived component of high-level nuclear wastes.
- Some 300 reactor-years experience has been gained in operating them
About 20 Fast Neutron Reactors have already been operating, some
since the 1950s, and some supply electricity commercially. Over 300
reactor-years of operating experience have been accumulated. These more
deliberately use the uranium-238 as well as the fissile U-235 isotope
used in most reactors. If they are designed to produce more plutonium
than they consume, they are called Fast Breeder Reactors (FBR). If they
are net consumers of plutonium they are sometimes called
"burners". Fast neutron reactors also can burn long-lived
actinides which are recovered from used fuel out of ordinary reactors.
Several countries have research and development programs for improved
Fast Neutron Reactors, and the IAEA's INPRO program involving 22
countries (see later section) has fast neutron reactors as a major
emphasis, in connection with closed fuel cycle. For instance one
scenario in France is for half of the present nuclear capacity to be
replaced by fast neutron reactors by 2050 (the first half being
replaced by 3rd-generation EPR units).
The FBR was originally conceived to extend the world's uranium
resources, and could do this by a factor of about 60. When those
resources were perceived to be scarce, several countries embarked upon
extensive FBR development programs. However significant technical and
materials problems were encountered, and also geological exploration
showed by the 1970s that scarcity was not going to be a concern for
some time. Due to both factors, by the 1980s it was clear that FBRs
would not be commercially competitive with existing light water
reactors.
Today there has been progress on the technical front, but the
economics of FBRs still depends on the value of the plutonium fuel
which is bred, relative to the cost of fresh uranium. Also there is
international concern over the disposal of ex-military plutonium, and
there are proposals to use fast reactors for this purpose. In both
respects the technology is important to long term considerations of
world energy sustainability.
see also American Nuclear Society position statement, November 2005 (pdf).
The fast reactor has no moderator and relies on fast neutrons alone
to cause fission, which is less efficient than using slow neutrons.
Hence a fast reactor uses plutonium or relatively highly-enriched
uranium (about 20% U-235) as its basic fuel, since it fissions
sufficiently with fast neutrons to keep going*. At the same time the
number of neutrons produced per fission is 25% more than from uranium,
and this means that there are enough (after losses) not only to
maintain the chain reaction but also to convert U-238 in a "fertile
blanket" around the core into fissile plutonium. No moderator is used
in the breeder reactor since fast neutrons are more efficient in
transmuting non-fissile U-238 in this "blanket" to Pu-239. The use of
liquid sodium as coolant avoids any neutron moderation and provides a
very efficient heat transfer medium. So, the fast reactor "burns" and
can "breed" plutonium.**
* high-enriched uranium would fission,
too. At this concentration of U-235, the cross-section for fission with
fast neutrons is sufficient to sustain the chain-reaction despite less
likelihood of fission, so about 20% of fissile nuclei is required in
the fuel. Up to 20% U is actually defined as "low-enriched' uranium.
** Both U-238 and Pu-240 are "fertile" (materials), i.e. by capturing a
neutron they become (directly or indirectly) fissile Pu-239 and Pu-241
respectively.
The core of a fast reactor is much smaller than that of a normal
nuclear reactor, and it has a higher power density, requiring very
efficient heat transfer. For instance, the core of Russia's BN-600
reactor (560 MWe) is 2 metres high and 0.75 m diameter. Fuel may be
enriched uranium oxide (BN-350, BN-600) or MOX (BOR-60, BN-800).
Both U-238 and Pu-240 are "fertile" (materials), i.e. by capturing a
neutron they become (directly or indirectly) fissile Pu-239 and Pu-241
respectively.
Natural uranium contains about 0.7% U-235 and 99.3% U-238. In any
reactor the U-238 component is turned into several isotopes of
plutonium during its operation. Two of these, Pu-239 and Pu-241, then
undergo fission in the same way as U-235 to produce heat. In a FBR this
process can be optimised so that it 'breeds' fuel, though reprocessing
of the blanket material is required to recover it. Hence FBRs can
utilise uranium at least 60 times more efficiently than a normal
reactor. They are however expensive to build and operate, including the
reprocessing, and could only be justified economically if uranium
prices were to rise to pre-1980 values in real terms.
One effect of this halt to FBR development is that separated
plutonium (from reprocessing used light water reactor fuel) which was
originally envisaged for FBRs is now being used as mixed oxide (MOX)
fuel in conventional reactors.
Fast neutron reactors have a high power density and are normally
cooled by liquid metal such as sodium, lead, or lead-bismuth, with high
conductivity and boiling point and no moderating effect. They operate
at around 500-550°C at or near atmospheric pressure. Fast reactors
typically use boron carbide control rods.
In some respects a liquid metal coolant is more benign overall than
very high pressure water, which requires robust engineering on account
of the pressure. However, the design needs to ensure that there is no
chemical interaction (eg sodium-water), and is lead-cooled, the
materials used need to allow for molten lead being very corrosive. Some
future plans are for gas-cooled fast reactors.
Also fast reactors have a strong negative temperature coefficient
(the reaction slows as the temperature rises unduly), an inherent
safety feature, and the basis of automatic load following in many new
designs.
Experiments on a 19-year old UK breeder reactor before it was
decommissioned in 1977, and on EBR-2 in the USA in 1986, showed that
the metal fuel with liquid sodium cooling system made them less
sensitive to coolant failures than the more conventional very high
pressure water and steam systems in light water reactors. More recent
operating experience with large French and UK prototypes has confirmed
this. With loss of coolant flow they simply shut themselves down.
There is renewed interest in fast reactors due to their ability to
fission actinides, including those which may be recovered from ordinary
reactor used fuel. The fast neutron environment minimises neutron
capture reactions and maximises fissions in actinides. This means less
long-lived nuclides in high-level wastes (the fission products being
preferable due to shorter lives).
Fast Neutron Reactors
| Output: |
MWe |
MW (thermal) |
Operation |
| USA |
| EBR 1 |
0.2 |
|
1951-63 |
| EBR 2 |
20 |
|
1963-94 |
| Fermi 1 |
66 |
|
1963-72 |
| SEFOR |
|
20 |
1969-72 |
| Fast Flux TF |
|
400 |
1980-93 |
| UK |
| Dounreay FR |
15 |
|
1959-77 |
| Protoype FR |
270 |
|
1974-94 |
| France |
| Rapsodie |
|
40 |
1966-82 |
| Phenix* |
250 |
|
1973- |
| Superphenix 1 |
1240 |
|
1985-98 |
| Germany |
| KNK 2 |
21 |
|
1977-91 |
| India |
| FBTR |
|
40 |
1985- |
| Japan |
| Joyo |
|
140 |
1978- |
| Monju |
280 |
|
1994-96-? |
| Kazakhstan |
| BN 350* |
135 |
|
1972-99 |
| Russia |
| BR 5 /10 |
|
5 /10 |
1959-71, 1973- |
| BOR 60 |
12 |
|
1969- |
| BN 600* |
560 |
|
1980- |
Europe, Russia, Kazakhstan
France has operated its Phenix fast reactor from 1973, apart from a few years for refurbishing. Closure of the 1250 MWe commercial prototype Superphenix FBR in
1998 on political grounds after very little operation over 13 years set
back developments. Research work on the 1450 MWe European FBR has
almost ceased.
The Russian BN-600
fast breeder reactor - Beloyarsk unit 3 - has been supplying
electricity to the grid since 1980 and is said to have the best
operating and production record of all Russia's nuclear power
units. It uses chiefly uranium oxide fuel, some enriched to over
20%, with some MOX in recent years. The sodium coolant delivers
550°C at little more than atmospheric pressure. Russia plans to
reconfigure the BN-600 by replacing the fertile blanket around the core
with steel reflector assemblies to burn the plutonium from its military
stockpiles and to extend its life beyond the 30 year design span.
The BN-350
prototype FBR generated power in Kazakhstan for 27 years to 1999 and
about half of its 1000 MW(thermal) output was used for water
desalination. It used uranium enriched to 17-26%. Its design life was
20 years, and after 1993 it operated on the basis of annual licence
renewal. Russia's BOR-60 was a demonstration model preceding it.
Construction has started on Beloyarsk-4 which is the first BN-800,
a new, more powerful (880 MWe) FBR, which is actually the same overall
size as BN-600. It has improved features including fuel
flexibility - U+Pu nitride, MOX, or metal, and with breeding ratio up
to 1.3. However, during the plutonium disposition campaign it will be
operated with a breeding ratio of less than one. It has much
enhanced safety and improved economy - operating cost is expected to be
only 15% more than VVER. It is capable of burning up to 2 tonnes
of plutonium per year from dismantled weapons and will test the
recycling of minor actinides in the fuel. Further BN-800 units
are planned.
Industry spokesmen had warned the government that Russia's world
leadership in FBR development was threatened due to lack of funding for
completion of BN-800, but this now seems to be resolved.
Russia has experimented with several lead-cooled reactor designs,
and has used lead-bismuth cooling for 40 years in reactors for its Alfa
class submarines. Pb-208 (54% of naturally-occurring lead) is
transparent to neutrons. A significant new Russian design is the BREST fast
neutron reactor, of 300 MWe or more with lead as the primary coolant,
at 540°C, and supercritical steam generators. It is inherently safe and
uses a U+Pu nitride fuel. No weapons-grade Pu can be produced (since
there is no uranium blanket), and spent fuel can be recycled
indefinitely, with on-site facilities. A pilot unit is being built at
Beloyarsk and 1200 MWe units are planned.
A smaller and newer Russian design is the Lead-Bismuth Fast Reactor (SVBR)
of 75-100 MWe. This is an integral design, with the steam generators
sitting in the same Pb-Bi pool at 400-480°C as the reactor core, which
could use a wide variety of fuels. The unit would be factory-made and
shipped as a 4.5m diameter, 7.5m high module, then installed in a tank
of water which gives passive heat removal and shielding. A power
station with 16 such modules is expected to supply electricity at lower
cost than any other new Russian technology as well as achieving
inherent safety and high proliferation resistance. (Russia built 7
Alfa-class submarines, each powered by a compact 155 MWt Pb-Bi cooled
reactor, and 70 reactor-years operational experience was acquired with
these.)
In the UK, the Dounreay Fast
Reactor started operating in 1959 using sodium-potassium coolant. This
was followed there by the much larger Prototype Fast Reactor which
operated for 20 years until the government withdrew funding.
Japan, India, China
A significant part of Japanese energy policy has been to develop
FBRs in order to improve uranium utilisation dramatically. From 1961 to
1994 there was a strong commitment to FBRs, but in 1994 the FBR
commercial timeline was pushed out to 2030, and in 2005 commercial FBRs
were envisaged by 2050.
In 1999 Japan Nuclear Cycle Development Institute (JNC) initiated a
program to review promising concepts, define a development plan by 2005
and establish a system of FBR technology by 2015. The parameters are:
passive safety, economic competitiveness with LWR, efficient
utilisation of resources (burning transuranics and depleted U), reduced
wastes, proliferation resistance and versatility (include hydrogen
production). Utilities are also involved.
Phase 2 of the study focused on four basic reactor designs:
sodium-cooled with MOX and metal fuels, helium-cooled with nitride and
MOX fuels, lead-bismuth eutectic-cooled with nitride and metal fuels,
and supercritical water-cooled with MOX fuel. All involve closed fuel
cycle, and three reprocessing routes were considered: advanced aqueous,
oxide electrowinning and metal pyroprocessing (electrorefining). This
work is linked with the Generation IV initiative, where Japan is
playing a leading role with sodium-cooled FBRs.
Japan's Joyo experimental reactor which has been operating since 1977 is now being boosted to 140 MWt.
The 280 MWe Monju prototype
FBR reactor started up in April 1994, but a sodium leakage in its
secondary heat transfer system during performance tests in 1995 meant
that it was shut down and has not operated since. It produced 246 MWe
when it was operating. Its oversight has passed to JNC, and the
Minister for Science & Technology has said that its early restart
is a key aim. A Supreme court decision in May 2005 cleared the way for
restarting it, probably in 2008.
Mitsubishi Heavy Industries (MHI) is involved with a consortium to build the Japan Standard Fast Reactor
(JSFR) concept, though with breeding ratio less than 1:1. This is
a large unit which will burn actinides with uranium and plutonium in
oxide fuel. It could be of any size from 500 to 1500 MWe.
In this connection MHI has also set up Mitsubishi FBR Systems (MFBR).
Japan's LSPR is
a lead-bismuth cooled reactor design of 150 MWt /53 MWe. Fuelled units
would be supplied from a factory and operate for 30 years, then be
returned. Concept intended for developing countries.
A small-scale design developed by Toshiba Corporation in cooperation
with Japan's Central Research Institute of Electric Power Industry
(CRIEPI) and funded by the Japan Atomic Energy Research Institute
(JAERI) is the 5 MWt, 200 kWe Rapid-L,
using lithium-6 (a liquid neutron poison) as control medium. It would
have 2700 fuel pins of 40-50% enriched uranium nitride with 2600°C
melting point integrated into a disposable cartridge. The reactivity
control system is passive, using lithium expansion modules (LEM) which
give burnup compensation, partial load operation as well as negative
reactivity feedback. As the reactor temperature rises, the lithium
expands into the core, displacing an inert gas. Other kinds of lithium
modules, also integrated into the fuel cartridge, shut down and start
up the reactor. Cooling is by molten sodium, and with the LEM control
system, reactor power is proportional to primary coolant flow rate.
Refuelling would be every 10 years in an inert gas environment.
Operation would require no skill, due to the inherent safety design
features. The whole plant would be about 6.5 metres high and 2 metres
diameter.
The Super-Safe, Small & Simple - 4S 'nuclear battery' system
is being developed by Toshiba and CRIEPI in Japan in collaboration with
STAR work in USA. It uses sodium as coolant (with electromagnetic
pumps) and has passive safety features, notably negative temperature
and void reactivity. The whole unit would be factory-built, transported
to site, installed below ground level, and would drive a steam cycle.
It is capable of three decades of continuous operation without
refuelling. Metallic fuel (169 pins 10mm diameter) is uranium-zirconium
or U-Pu-Zr alloy enriched to less than 20%. Steady power output over
the core lifetime is achieved by progressively moving upwards an
annular reflector around the slender core (0.68m diameter, 2m high).
After 14 years a neutron absorber at the centre of the core is removed
and the reflector repeats its slow movement up the core for 16 more
years. In the event of power loss the reflector falls to the bottom of
the reactor vessel, slowing the reaction, and external air circulation
gives decay heat removal.
Both 10 MWe and 50 MWe versions of 4S are designed to automatically
maintain an outlet coolant temperature of 510°C - suitable for power
generation with high temperature electrolytic hydrogen production.
Plant cost is projected at US$ 2500/kW and power cost 5-7 cents/kWh for
the small unit - very competitive with diesel in many locations. The
design has gained considerable support in Alaska and and toward the end
of 2004 the town of Galena granted initial approval for Toshiba to
build a 4S reactor in that remote location. A pre-application NRC
review is being sought with a view to a demonstration unit operating by
2012. Its design is sufficiently similar to PRISM -
GE's modular 150 MWe liquid metal-cooled inherently-safe reactor which
went part-way through US NRC approval process for it to have good
prospects of licensing.
The L-4S is Pb-Bi cooled version of 4S.
In India, research continues. At the Indira Gandhi Centre for Atomic Research a 40 MWt fast breeder test reactor (FBTR) has been operating since 1985. In addition, the tiny Kamini there is employed to explore the use of thorium as nuclear fuel, by breeding fissile U-233.
In 2002 the regulatory authority issued approval to start construction of a 500 MWe prototype fast breeder reactor (PFBR) at Kalpakkam and
this is now under construction by BHAVINI. It is expected to be
operating in 2010, fuelled with uranium-plutonium oxide (the
reactor-grade Pu being from its existing PHWRs) and with a thorium
blanket to breed fissile U-233. This will take India's ambitious
thorium program to stage 2, and set the scene for eventual full
utilisation of the country's abundant thorium to fuel reactors. Four
more such fast reactors have been announced for construction by 2020.
Initial Indian FBRs will be have mixed oxide fuel but these will be
followed by metallic-fuelled ones to enable shorter doubling time.
In China, a 65 MWt fast neutron reactor - the Chinese Experimental Fast Reactor (CEFR)
- is under construction near Beijing and due to achieve criticality in
2008. There has been some Russian assistance in its development.
R&D on fast neutron reactors started in 1964. A 600 MWe prototype
fast reactor is envisaged by 2020 and there is talk of a 1500 MWe one
by 2030. CNNC expects the technology to become predominant by mid
century.
USA
In the USA, five fast neutron reactors have operated, and several more designed. The experimental breeder reactor EBR-1 at Idaho in 1951 produced enough power to run its own building - a milestone achievement.
The EBR-2 was
a demonstration reactor - 62.5 MW thermal, and it typically operated at
19 MWe, providing heat and power to the Idaho facility. The idea was to
demonstrate a complete sodium-cooled breeder reactor power plant with
on-site reprocessing of metallic fuel, an this was successfully done
1964-69. The emphasis then shifted to testing materials and fuels
(metal and ceramic oxides, carbides and nitrides of U & Pu) for
larger fast reactors. Finally it became the IFR prototype, using
metallic alloy U-Pu-Zr fuels. All the time, it generated some 1 TWh of
power as well.
The EBR-2 was integral to the US Integral Fast Reactor (IFR)
program, considered by the National Academy of Sciences to be the
nation's highest priority research for future reactor types. This was
developing a fully-integrated system with pyro-reprocessing, fuel
fabrication and fast reactor in same complex. The reactor could be
operated as a breeder or not. Some $46 million of the IFR funding was
provided by a Japanese utility consortium.
IFR program goals were demonstrating inherent safety apart from
engineered controls, improved management of high-level nuclear wastes
by recycling all actinides, so that only fission products remain as
HLW, and using the full energy potential of uranium rather than only
about one percent of it. All these were demonstrated, though the
program was aborted before the recycle of neptunium and americium was
properly evaluated. IFR fuel first used in 1986 reached 19% burnup
(compared with 3-4% for conventional reactors), and 22% was targeted.
A further political goal was demonstrating a proliferation-resistant
closed fuel cycle, with plutonium being recycled with other actinides.
In 1994, Congress under the Clinton administration shut EBR-2 down.
The IFR program is now being reinvented as part of the Global Nuclear
Energy Partnership (see below), while EBR-2 is being decommissioned. An
EBR-3 of 200-300 MWe was proposed but not developed.
The first US commercial FBR was Fermi-1 in
Michigan, but it operated for only three years before a coolant problem
caused overheating and it was shut down with some damage to the fuel.
After repair it was restarted in 1970, but its licence was not renewed
in 1972.
The Southeast Experimental Fast Oxide Reactor (SEFOR)
was built in 1965 and operated for three years in Arkansas by GE under
contract to the US government. It was the only fast reactor to use a
full core of Pu-U mixed oxide fuel, and was sodium-cooled. It
completed its safety test program in 1972, demonstrating the capability
of the Doppler coefficient (re core thermal expansion) in a mixed oxide
reactor to stabilise it and control accidents in oxide-fueled,
sodium-cooled fast reactors. Fuel and coolant were removed in
1972 and the University of Arkansas bought it in 1975.
The 400 MWt Fast Flux Test Facility
was in full operation 1982-92 at Hanford as a major national research
reactor. It was closed down at the end of 1993, and since 2001 it has
been deactivated under care and maintenance pending possible
decommissioning. However, in August 2006 the Department of Energy
indicated that it could possibly be recommissioned as part of the
Global Nuclear Energy Partnership demonstration process.
GE with the DOE national laboratories has been developing a modular liquid metal-cooled inherently-safe reactor - PRISM
during the advanced liquid-metal fast breeder reactor (ALMR)
program. No US fast neutron reactor has so far been larger than
66 MWe and none has supplied electricity commercially.
Today's PRISM
is a GE-Hitachi design for compact modular pool-type reactors with
passive cooling for decay heat removal. After 30 years of
development it represents GEH's Generation IV solution to closing the
fuel cycle in the USA. Modules are 200 to 360 MWe and operate at
high temperature - over 500∞C. The pool-type modules contain the
complete primary system with sodium coolant. The Pu & DU fuel
is metal, and obtained from used light water reactor fuel.
However, all transuranic elements are removed together in the
electrometallurgical reprocessing so that fresh fuel has minor
actinides with the plutonium. Fuel stays in the reactor about six
years, with one third removed every two years. The
commercial-scale plant concept uses six reactor modules to provide 1200
to 2200 MWe.
The Encapsulated Nuclear Heat Source (ENHS)
concept is a liquid metal-cooled reactor of 50 MWe being developed by
the University of California. The core is in a metal-filled module
sitting in a large pool of secondary molten metal coolant which also
accommodates the separate and unconnected steam generators. Fuel is a
uranium-zirconium alloy with 13% U enrichment (or U-Pu-Zr with 11% Pu)
with a 15-year life. After this the module is removed, stored on site
until the primary lead (or Pb-Bi) coolant solidifies, and it would then
be shipped as a self-contained and shielded item. A new fuelled module
would be supplied complete with primary coolant. The ENHS is designed
for developing countries but is not yet close to commercialisation.
A related project is the Secure Transportable Autonomous Reactor - STAR
being developed by Argonne under the leadership of Lawrence Livermore
Laboratory (DOE). It is a lead-cooled fast neutron modular reactor with
passive safety features. Its 400 MWt. size means it can be shipped by
rail and cooled by natural circulation. It uses U-transuranic nitride
fuel in a cassette which is replaced every 15-20 years. The STAR-LM was
conceived for power generation, running at 578°C and producing 180 MWe.
The STAR-LM was conceived for power generation, running at 578°C and producing 180 MWe.
STAR-H2 is an
adaptation for hydrogen production, with reactor heat at up to 800°C
being conveyed by a helium circuit to drive a separate thermochemical
hydrogen production plant, while lower grade heat is harnessed for
desalination (multi-stage flash process). Any commercial electricity
generation then would be by fuel cells, from the hydrogen. Its
development is further off.
A smaller STAR variant is the Small Sealed Transportable Autonomous Reactor - SSTAR,
being developed in collaboration with Toshiba and others in Japan (see
4S below). It has lead or Pb-Bi cooling, runs at 566°C and has integral
steam generator inside the sealed unit, which would be installed below
ground level. Conceived in sizes 10-100 MWe, main development is now
focused on a 45 MWt/ 20 MWe version as part of the US Generation IV
effort. After a 20-year life without refuelling, the whole reactor unit
is then returned for recycling the fuel. The core is one metre diameter
and 0.8m high. SSTAR will eventually be coupled to a Brayton cycle
turbine using supercritical carbon dioxide. Prototype envisaged 2015.
For all STAR concepts, regional fuel cycle support centres would
handle fuel supply and reprocessing, and fresh fuel would be spiked
with fission products to deter misuse. Complete burnup of uranium and
transuranics is envisaged in STAR-H2, with only fission products being
waste.
Generation IV fast reactors
In 2003 the Generation IV International Forum (GIF) representing ten
countries announced the selection of six reactor technologies which
they believe represent the future shape of nuclear energy. These were
selected on the basis of being clean, safe and cost-effective means of
meeting increased energy demands on a sustainable basis, while being
resistant to diversion of materials for weapons proliferation and
secure from terrorist attacks. They will be the subject of further
development internationally. Led by the USA, Argentina, Brazil, Canada,
France, Japan, South Korea, South Africa, Switzerland, and the UK are
members of the GIF, along with the EU. India has applied to join.
Most of the six systems employ a closed fuel cycle to maximise the
resource base and minimise high-level wastes to be sent to a
repository. Three of the six are fast reactors and one can be built as
a fast reactor, one is described as epithermal - these five are
described below. Only two operate with slow neutrons like today's
plants.
Of the five, only one is cooled by light water, one is helium-cooled
and the others have lead-bismuth, sodium or fluoride salt coolant. The
latter three operate at low pressure, with significant safety
advantage. The last has the uranium fuel dissolved in the circulating
coolant. Temperatures range from 510°C to 850°C, compared with less
than 330°C for today's light water reactors, and this means that three
of them can be used for thermochemical hydrogen production.
The sizes range from 150 to 1500 MWe (or equivalent thermal) , with
the lead-cooled one optionally available as a 50-150 MWe "battery" with
long core life (15-20 years without refuelling) as replaceable cassette
or entire reactor module. This is designed for distributed generation
or desalination.
At least three of the five systems have significant operating
experience already in most respects of their design, which may mean
that they can be in commercial operation well before 2030.
In February 2005 five of the participants signed an agreement to
take forward the R&D on the six technologies. The USA, Canada,
France, Japan and UK agreed to undertake joint research and exchange
technical information.
While Russia is not a part of GIF, one design corresponds with the
BREST reactor being developed there, and Russia is now the main
operator of the sodium-cooled fast reactor for electricity - another of
the technologies put forward by the GIF:
Gas-cooled fast reactors. Like
other helium-cooled reactors which have operated or are under
development, these will be high-temperature units - 850°C, suitable for
power generation, thermochemical hydrogen production or other process
heat. For electricity, the gas will directly drive a gas turbine
(Brayton cycle). Fuels would include depleted uranium and any other
fissile or fertile materials. Spent fuel would be reprocessed on site
and all the actinides recycled to minimise production of long-lived
radioactive wastes.
While General Atomics worked on the design in the 1970s (but not as fast reactor), none has so far been built.
Lead-cooled fast reactors.
Liquid metal (Pb or Pb-Bi) cooling is by natural convection. Fuel is
depleted uranium metal or nitride, with full actinide recycle from
regional or central reprocessing plants. A wide range of unit sizes is
envisaged, from factory-built "battery" with 15-20 year life for small
grids or developing countries such as teh SSTAR described above, to
modular 300-400 MWe units and large single plants of 1400 MWe.
Operating temperature of 550°C is readily achievable but 800°C is
envisaged with advanced materials and this would enable thermochemical
hydrogen production.
This corresponds with Russia's BREST fast reactor technology which
is lead-cooled and builds on 40 years experience of lead-bismuth
cooling in submarine reactors. Its fuel is U+Pu nitride. More
immediately the GIF proposal appears to arise from two experimental
designs: the US STAR and Japan's LSPR, these being lead and
lead-bismuth cooled respectively.
Sodium-cooled fast reactors.
This builds on more than 300 reactor-years experienced with fast
neutron reactors over five decades and in eight countries. It utilises
depleted uranium in the fuel and has a coolant temperature of 550°C
enabling electricity generation via a secondary sodium circuit, the
primary one being at near atmospheric pressure. Two variants were
proposed: a 150-500 MWe type with actinides incorporated into a metal
fuel requiring pyrometallurgical processing on site, and a 500-1500 MWe
type with conventional MOX fuel reprocessed in conventional facilities
elsewhere. In the light of the GNEP announcement in 2006, the latter
course looks less likely.
In 2008 France, Japan and the USA have signed two agreements to
collaborate on developing sodium-cooled fast reactors. These are
initially focused on using Phenix until it shuts down in 2009, then on
Japan's Monju, and extends to aspects of fuel cycle. The work
will involve demonstrating transmutation in connection with the Global
Actinide Cycle International Demonstration (GACID) program, led by
France. Beyond using Monju, the French CEA, the Japan Atomic
Energy Agency and the US DOE have been discussing the size of planned
prototypes, reactor types, fuel types, and schedules for
deployment. The CEA has begun design of a prototype sodium fast
reactor of 250 to 600 MWe, SFR, planned to operate in 2020.
Supercritical water-cooled reactors.
This is a very high-pressure water-cooled reactor which operates above
the thermodynamic critical point of water to give a thermal efficiency
about one third higher than today's light water reactors from which the
design evolves. The supercritical water (25 MPa and 510-550°C) directly
drives the turbine, without any secondary steam system. Passive safety
features are similar to those of simplified boiling water reactors.
Fuel is uranium oxide, enriched in the case of the open fuel cycle
option. However, it can be built as a fast reactor with full actinide
recycle based on conventional reprocessing. Most research on the design
has been in Japan.
Molten salt reactors. While
not strictly a fast neutron reactor, the uranium fuel is dissolved in
the sodium fluoride salt coolant which circulates through graphite core
channels to achieve some moderation and an epithermal neutron spectrum.
Fission products are removed continuously and the actinides are fully
recycled, while plutonium and other actinides can be added along with
U-238. Coolant temperature is 700°C at very low pressure, with 800°C
envisaged. A secondary coolant system is used for electricity
generation, and thermochemical hydrogen production is also feasible.
During the 1960s the USA developed the molten salt breeder reactor
as the primary back-up option for the conventional fast breeder reactor
and a small prototype was operated. Recent work has focused on lithium
and beryllium fluoride coolant with dissolved thorium and U-233 fuel.
The attractive features of the MSR fuel cycle include: the high-level
waste comprising fission products only, hence shorter-lived
radioactivity; small inventory of weapons-fissile material (Pu-242
being the dominant Pu isotope); low fuel use (the French self-breeding
variant claims 50kg of thorium and 50kg U-238 per billion kWh); and
safety due to passive cooling up to any size.
INPRO
As well as the GIF, another program with similar aims is coordinated
by the IAEA. This is the International Project on Innovative Nuclear
Reactors and Fuel Cycles (INPRO). It was launched in 2001 and has 22
members including Russia, aiming "to support the safe, sustainable,
economic and proliferation-resistant use of nuclear technology to meet
the global energy needs of the 21st century." It does this by examining
issues related to the development and deployment of Innovative Nuclear
Energy Systems (INS) for sustainable energy supply.
One of the case studies in phase 1 of INPRO was undertaken by Russia on its BN-800
fast reactor, though the emphasis was on the methodology rather than
the technology. Nevertheless, fast reactor systems will feature in
further INPRO work.
Global Nuclear Energy Partnership (GNEP)
This concept, announced in 2006, builds on earlier US work with the
Integral Fast Reactor (IFR) project and international work on fast
reactors. Its main thrust in to counter proliferation concerns, but
will have the effect of much greater resource utilisation as well.
It envisages fabrication and leasing of fuel for conventional
reactors, with the used fuel being returned to fuel supplier countries
and pyro-processed to recover uranium and actinides, leaving only
fission products as high-level waste. The actinide mix is then burned
in on-site fast reactors.
Physics of fast neutron reactors
In an idealised Fast Neutron Reactor the fuel in the core is Pu-239
and the abundant neutrons designed to leak from the core would breed
more Pu-239 in the fertile blanket of U-238 around the core. A minor
fraction of U-238 might be subject to fission, but most of the neutrons
reaching the U-238 blanket will have lost some of their original energy
and are therefore subject only to capture and the eventual generation
of Pu-239. Cooling of the fast reactor core requires a heat transfer
medium which has minimal moderation of the neutrons, and hence liquid
metals are used, typically sodium or a mixture of sodium and potassium.
Such reactors are more efficient at converting fertile material than
ordinary thermal reactors because of the arrangement of fissile and
fertile materials, and there is some advantage from the fact that
Pu-239 yields more neutrons per fission than U-235. Although both yield
more neutrons per fission when split by fast rather than slow neutrons,
this is incidental since the fission cross sections are much smaller at
high neutron energies. Fast neutron reactors may be designed as
breeders to yield more fissile material than they consume or to be
plutonium burners to dispose of excess plutonium. A plutonium burner
would be designed without a breeding blanket, simply with a core
optimised for plutonium fuel.
References:
other WNA briefing/information papers
IAEA Fast Reactors database
ANS position paper: www.ans.org/pi/ps/docs/ps74.pdf
IFR web site: www.nuc.berkeley.edu/designs/ifr